An approach for patterned molecular adsorption on ferromagnets, achieved via Moiré superstructures

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An approach for patterned molecular adsorption on ferromagnets, achieved via Moiré superstructures. / Jensen, Sigmund; Løge, Isaac Appelquist; Bendix, Jesper; Diekhöner, Lars.

I: Physical Chemistry Chemical Physics, 2024.

Publikation: Bidrag til tidsskrift › Tidsskriftartikel › Forskning › fagfællebedømt

Harvard

Jensen, S, Løge, IA, Bendix, J & Diekhöner, L 2024, 'An approach for patterned molecular adsorption on ferromagnets, achieved via Moiré superstructures', Physical Chemistry Chemical Physics. https://doi.org/10.1039/d4cp00809j

APA

Jensen, S., Løge, I. A., Bendix, J., & Diekhöner, L. (Accepteret/In press). An approach for patterned molecular adsorption on ferromagnets, achieved via Moiré superstructures. Physical Chemistry Chemical Physics. https://doi.org/10.1039/d4cp00809j

Vancouver

Jensen S, Løge IA, Bendix J, Diekhöner L. An approach for patterned molecular adsorption on ferromagnets, achieved via Moiré superstructures. Physical Chemistry Chemical Physics. 2024. https://doi.org/10.1039/d4cp00809j

Author

Jensen, Sigmund ; Løge, Isaac Appelquist ; Bendix, Jesper ; Diekhöner, Lars. / An approach for patterned molecular adsorption on ferromagnets, achieved via Moiré superstructures. I: Physical Chemistry Chemical Physics. 2024.

Bibtex

@article{bdc34d2a193342fa903792213f1fec7b,
title = "An approach for patterned molecular adsorption on ferromagnets, achieved via Moir{\'e} superstructures",
abstract = "We have used a scanning tunneling microscope operated under ultrahigh vacuum conditions to investigate an oxo-vanadium-salen complex V(O)salen, that has potential applications as qubits in future quantum-based technologies. The adsorption and self-assembly of V(O)salen on a range of single crystal metal surfaces and nanoislands and the influence of substrate morphology and reactivity has been measured. On the close-packed flat Ag(111) and Cu(111) surfaces, the molecules adsorb isolated or form small clusters arranged randomly on the surface, whereas structured adsorption occurs on two types of Co nanoislands; Co grown on Ag(111) and Ag capped Co islands grown on Cu(111), both forming a Moir{\'e} pattern at the surface. The adsorption configuration can by scanning tunneling spectroscopy be linked to the geometric and electronic properties of the substrates and traced back to a Co d-related surface state, illustrating how the modulated reactivity can be used to engineer a pattern of adsorbed molecules on the nanoscale.",
author = "Sigmund Jensen and L{\o}ge, {Isaac Appelquist} and Jesper Bendix and Lars Diekh{\"o}ner",
note = "Publisher Copyright: {\textcopyright} 2024 The Royal Society of Chemistry.",
year = "2024",
doi = "10.1039/d4cp00809j",
language = "English",
journal = "Physical Chemistry Chemical Physics",
issn = "1463-9076",
publisher = "Royal Society of Chemistry",

}

RIS

TY - JOUR

T1 - An approach for patterned molecular adsorption on ferromagnets, achieved via Moiré superstructures

AU - Jensen, Sigmund

AU - Løge, Isaac Appelquist

AU - Bendix, Jesper

AU - Diekhöner, Lars

N1 - Publisher Copyright: © 2024 The Royal Society of Chemistry.

PY - 2024

Y1 - 2024

N2 - We have used a scanning tunneling microscope operated under ultrahigh vacuum conditions to investigate an oxo-vanadium-salen complex V(O)salen, that has potential applications as qubits in future quantum-based technologies. The adsorption and self-assembly of V(O)salen on a range of single crystal metal surfaces and nanoislands and the influence of substrate morphology and reactivity has been measured. On the close-packed flat Ag(111) and Cu(111) surfaces, the molecules adsorb isolated or form small clusters arranged randomly on the surface, whereas structured adsorption occurs on two types of Co nanoislands; Co grown on Ag(111) and Ag capped Co islands grown on Cu(111), both forming a Moiré pattern at the surface. The adsorption configuration can by scanning tunneling spectroscopy be linked to the geometric and electronic properties of the substrates and traced back to a Co d-related surface state, illustrating how the modulated reactivity can be used to engineer a pattern of adsorbed molecules on the nanoscale.

AB - We have used a scanning tunneling microscope operated under ultrahigh vacuum conditions to investigate an oxo-vanadium-salen complex V(O)salen, that has potential applications as qubits in future quantum-based technologies. The adsorption and self-assembly of V(O)salen on a range of single crystal metal surfaces and nanoislands and the influence of substrate morphology and reactivity has been measured. On the close-packed flat Ag(111) and Cu(111) surfaces, the molecules adsorb isolated or form small clusters arranged randomly on the surface, whereas structured adsorption occurs on two types of Co nanoislands; Co grown on Ag(111) and Ag capped Co islands grown on Cu(111), both forming a Moiré pattern at the surface. The adsorption configuration can by scanning tunneling spectroscopy be linked to the geometric and electronic properties of the substrates and traced back to a Co d-related surface state, illustrating how the modulated reactivity can be used to engineer a pattern of adsorbed molecules on the nanoscale.

U2 - 10.1039/d4cp00809j

DO - 10.1039/d4cp00809j

M3 - Journal article

C2 - 38669006

AN - SCOPUS:85191325757

JO - Physical Chemistry Chemical Physics

JF - Physical Chemistry Chemical Physics

SN - 1463-9076

ER -

ID: 391035551