All-Inorganic Zero-Dimensional Sb3+-Doped Rb2ScCl5(H2O) Perovskite Single Crystals: Efficient Self-Trapped Exciton Emission and X-ray Detection

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Standard

All-Inorganic Zero-Dimensional Sb3+-Doped Rb2ScCl5(H2O) Perovskite Single Crystals : Efficient Self-Trapped Exciton Emission and X-ray Detection. / Mao, Xin; Wang, Zhongyi; Zhang, Fen; Yin, Hong; Xu, Xin; Chen, Junsheng; Chen, Zhen; Luo, Junhua; Han, Keli; Zhang, Ruiling.

I: Journal of Physical Chemistry Letters, Bind 14, Nr. 6, 2023, s. 1521-1527.

Publikation: Bidrag til tidsskrift › Tidsskriftartikel › Forskning › fagfællebedømt

Harvard

Mao, X, Wang, Z, Zhang, F, Yin, H, Xu, X, Chen, J, Chen, Z, Luo, J, Han, K & Zhang, R 2023, 'All-Inorganic Zero-Dimensional Sb3+-Doped Rb2ScCl5(H2O) Perovskite Single Crystals: Efficient Self-Trapped Exciton Emission and X-ray Detection', Journal of Physical Chemistry Letters, bind 14, nr. 6, s. 1521-1527. https://doi.org/10.1021/acs.jpclett.2c03912

APA

Mao, X., Wang, Z., Zhang, F., Yin, H., Xu, X., Chen, J., Chen, Z., Luo, J., Han, K., & Zhang, R. (2023). All-Inorganic Zero-Dimensional Sb3+-Doped Rb2ScCl5(H2O) Perovskite Single Crystals: Efficient Self-Trapped Exciton Emission and X-ray Detection. Journal of Physical Chemistry Letters, 14(6), 1521-1527. https://doi.org/10.1021/acs.jpclett.2c03912

Vancouver

Mao X, Wang Z, Zhang F, Yin H, Xu X, Chen J o.a. All-Inorganic Zero-Dimensional Sb3+-Doped Rb2ScCl5(H2O) Perovskite Single Crystals: Efficient Self-Trapped Exciton Emission and X-ray Detection. Journal of Physical Chemistry Letters. 2023;14(6):1521-1527. https://doi.org/10.1021/acs.jpclett.2c03912

Author

Mao, Xin ; Wang, Zhongyi ; Zhang, Fen ; Yin, Hong ; Xu, Xin ; Chen, Junsheng ; Chen, Zhen ; Luo, Junhua ; Han, Keli ; Zhang, Ruiling. / All-Inorganic Zero-Dimensional Sb3+-Doped Rb2ScCl5(H2O) Perovskite Single Crystals : Efficient Self-Trapped Exciton Emission and X-ray Detection. I: Journal of Physical Chemistry Letters. 2023 ; Bind 14, Nr. 6. s. 1521-1527.

Bibtex

@article{5af38b9874334411b2ea221bbb052efb,
title = "All-Inorganic Zero-Dimensional Sb3+-Doped Rb2ScCl5(H2O) Perovskite Single Crystals: Efficient Self-Trapped Exciton Emission and X-ray Detection",
abstract = "Zero-dimensional (0D) halide perovskites have attracted extensive attention for their potential applications in solid-state lighting and X-ray detection due to their fascinating optoelectronic properties and convenient solution processability. Herein, we report the synthesis and photophysical properties of high-quality Sb3+-doped 0D Rb2ScCl5(H2O) perovskite single crystals. The pristine crystals exhibit weak yellow self-trapped exciton (STE) emission peaking at 632 nm. The emission quantum yield can be dramatically enhanced from less than 1% to about 53% via Sb3+ doping. Spectroscopic characterizations indicate that the photoluminescence enhancement is a result of the efficient energy transfer from Sb3+ to the emissive STEs. Additionally, 0.2%Sb3+:Rb2ScCl5(H2O) single crystals exhibit potential application in direct X-ray detection with a high sensitivity of 58.5 μC Gy-1 cm-2",
author = "Xin Mao and Zhongyi Wang and Fen Zhang and Hong Yin and Xin Xu and Junsheng Chen and Zhen Chen and Junhua Luo and Keli Han and Ruiling Zhang",
note = "Funding Information: This work was supported by a project funded by the National Natural Science Foundation of China (Grant No. 22103050). Publisher Copyright: {\textcopyright} 2023 American Chemical Society.",
year = "2023",
doi = "10.1021/acs.jpclett.2c03912",
language = "English",
volume = "14",
pages = "1521--1527",
journal = "Journal of Physical Chemistry Letters",
issn = "1948-7185",
publisher = "American Chemical Society",
number = "6",

}

RIS

TY - JOUR

T1 - All-Inorganic Zero-Dimensional Sb3+-Doped Rb2ScCl5(H2O) Perovskite Single Crystals

T2 - Efficient Self-Trapped Exciton Emission and X-ray Detection

AU - Mao, Xin

AU - Wang, Zhongyi

AU - Zhang, Fen

AU - Yin, Hong

AU - Xu, Xin

AU - Chen, Junsheng

AU - Chen, Zhen

AU - Luo, Junhua

AU - Han, Keli

AU - Zhang, Ruiling

N1 - Funding Information: This work was supported by a project funded by the National Natural Science Foundation of China (Grant No. 22103050). Publisher Copyright: © 2023 American Chemical Society.

PY - 2023

Y1 - 2023

N2 - Zero-dimensional (0D) halide perovskites have attracted extensive attention for their potential applications in solid-state lighting and X-ray detection due to their fascinating optoelectronic properties and convenient solution processability. Herein, we report the synthesis and photophysical properties of high-quality Sb3+-doped 0D Rb2ScCl5(H2O) perovskite single crystals. The pristine crystals exhibit weak yellow self-trapped exciton (STE) emission peaking at 632 nm. The emission quantum yield can be dramatically enhanced from less than 1% to about 53% via Sb3+ doping. Spectroscopic characterizations indicate that the photoluminescence enhancement is a result of the efficient energy transfer from Sb3+ to the emissive STEs. Additionally, 0.2%Sb3+:Rb2ScCl5(H2O) single crystals exhibit potential application in direct X-ray detection with a high sensitivity of 58.5 μC Gy-1 cm-2

AB - Zero-dimensional (0D) halide perovskites have attracted extensive attention for their potential applications in solid-state lighting and X-ray detection due to their fascinating optoelectronic properties and convenient solution processability. Herein, we report the synthesis and photophysical properties of high-quality Sb3+-doped 0D Rb2ScCl5(H2O) perovskite single crystals. The pristine crystals exhibit weak yellow self-trapped exciton (STE) emission peaking at 632 nm. The emission quantum yield can be dramatically enhanced from less than 1% to about 53% via Sb3+ doping. Spectroscopic characterizations indicate that the photoluminescence enhancement is a result of the efficient energy transfer from Sb3+ to the emissive STEs. Additionally, 0.2%Sb3+:Rb2ScCl5(H2O) single crystals exhibit potential application in direct X-ray detection with a high sensitivity of 58.5 μC Gy-1 cm-2

U2 - 10.1021/acs.jpclett.2c03912

DO - 10.1021/acs.jpclett.2c03912

M3 - Journal article

C2 - 36745062

AN - SCOPUS:85147822656

VL - 14

SP - 1521

EP - 1527

JO - Journal of Physical Chemistry Letters

JF - Journal of Physical Chemistry Letters

SN - 1948-7185

IS - 6

ER -

ID: 339257527