2022 roadmap on low temperature electrochemical CO2 reduction

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  • Ifan E. L. Stephens
  • Karen Chan
  • Shannon W. Boettcher
  • Julien Bonin
  • Etienne Boutin
  • Aya K. Buckley
  • Raffaella Buonsanti
  • Etosha R. Cave
  • Xiaoxia Chang
  • See Wee Chee
  • Alisson H. M. da Silva
  • Phil de Luna
  • Oliver Einsle
  • Balazs Endrodi
  • Jorge V. Ferreira de Araujo
  • Marta C. Figueiredo
  • Christopher Hahn
  • Kentaro U. Hansen
  • Sophia Haussener
  • Sara Hunegnaw
  • Ziyang Huo
  • Yun Jeong Hwang
  • Csaba Janaky
  • Buddhinie S. Jayathilake
  • Feng Jiao
  • Zarko P. Jovanov
  • Parisa Karimi
  • Marc T. M. Koper
  • Kendra P. Kuhl
  • Woong Hee Lee
  • Zhiqin Liang
  • Xuan Liu
  • Sichao Ma
  • Ming Ma
  • Hyung-Suk Oh
  • Marc Robert
  • Beatriz Roldan Cuenya
  • Claudie Roy
  • Mary P. Ryan
  • Edward H. Sargent
  • Brian Seger
  • Ludmilla Steier
  • Peter Strasser
  • Ana Sofia Varela
  • Rafael E. Vos
  • Xue Wang
  • Bingjun Xu
  • Hossein Yadegari
  • Yuxiang Zhou

Electrochemical CO2 reduction (CO2R) is an attractive option for storing renewable electricity and for the sustainable production of valuable chemicals and fuels. In this roadmap, we review recent progress in fundamental understanding, catalyst development, and in engineering and scale-up. We discuss the outstanding challenges towards commercialization of electrochemical CO2R technology: energy efficiencies, selectivities, low current densities, and stability. We highlight the opportunities in establishing rigorous standards for benchmarking performance, advances in in operando characterization, the discovery of new materials towards high value products, the investigation of phenomena across multiple-length scales and the application of data science towards doing so. We hope that this collective perspective sparks new research activities that ultimately bring us a step closer towards establishing a low- or zero-emission carbon cycle.

OriginalsprogEngelsk
Artikelnummer042003
TidsskriftJPhys Energy
Vol/bind4
Udgave nummer4
Antal sider84
ISSN2515-7655
DOI
StatusUdgivet - 1 okt. 2022

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