Direct Writing of Room Temperature Polariton Condensate Lattice
Publikation: Bidrag til tidsskrift › Tidsskriftartikel › Forskning › fagfællebedømt
Standard
Direct Writing of Room Temperature Polariton Condensate Lattice. / Yadav, Ravindra Kumar; Satapathy, Sitakanta; Deshmukh, Prathmesh; Datta, Biswajit; Sharma, Addhyaya; Olsson, Andrew H.; Chen, Junsheng; Laursen, Bo W.; Flood, Amar H.; Sfeir, Matthew Y.; Menon, Vinod M.
I: Nano Letters, 2024.Publikation: Bidrag til tidsskrift › Tidsskriftartikel › Forskning › fagfællebedømt
Harvard
APA
Vancouver
Author
Bibtex
}
RIS
TY - JOUR
T1 - Direct Writing of Room Temperature Polariton Condensate Lattice
AU - Yadav, Ravindra Kumar
AU - Satapathy, Sitakanta
AU - Deshmukh, Prathmesh
AU - Datta, Biswajit
AU - Sharma, Addhyaya
AU - Olsson, Andrew H.
AU - Chen, Junsheng
AU - Laursen, Bo W.
AU - Flood, Amar H.
AU - Sfeir, Matthew Y.
AU - Menon, Vinod M.
N1 - Publisher Copyright: © 2024 American Chemical Society
PY - 2024
Y1 - 2024
N2 - Realizing lattices of exciton polariton condensates has been of much interest owing to the potential of such systems to realize analogue Hamiltonian simulators and physical computing architectures. Here, we report the realization of a room temperature polariton condensate lattice using a direct-write approach. Polariton condensation is achieved in a microcavity embedded with host-guest Frenkel excitons of an organic dye (rhodamine) in a small-molecule ionic isolation lattice (SMILES). The microcavity is patterned using focused ion beam etching to realize arbitrary lattice geometries, including defect sites on demand. The band structure of the lattice and the emergence of condensation are imaged using momentum-resolved spectroscopy. The introduction of defect sites is shown to lower the condensation threshold and result in the formation of a defect band in the condensation spectrum. The present approach allows us to study periodic, quasiperiodic, and disordered polariton condensate lattices at room temperature using a direct-write approach.
AB - Realizing lattices of exciton polariton condensates has been of much interest owing to the potential of such systems to realize analogue Hamiltonian simulators and physical computing architectures. Here, we report the realization of a room temperature polariton condensate lattice using a direct-write approach. Polariton condensation is achieved in a microcavity embedded with host-guest Frenkel excitons of an organic dye (rhodamine) in a small-molecule ionic isolation lattice (SMILES). The microcavity is patterned using focused ion beam etching to realize arbitrary lattice geometries, including defect sites on demand. The band structure of the lattice and the emergence of condensation are imaged using momentum-resolved spectroscopy. The introduction of defect sites is shown to lower the condensation threshold and result in the formation of a defect band in the condensation spectrum. The present approach allows us to study periodic, quasiperiodic, and disordered polariton condensate lattices at room temperature using a direct-write approach.
KW - condensate lattice
KW - molecular polaritons
KW - polariton
KW - polariton condensation
KW - polariton lattice
U2 - 10.1021/acs.nanolett.4c00586
DO - 10.1021/acs.nanolett.4c00586
M3 - Journal article
C2 - 38598721
AN - SCOPUS:85190154185
JO - Nano Letters
JF - Nano Letters
SN - 1530-6984
ER -
ID: 388947924