Quadrupole moments of Cd and Zn nuclei: When solid-state, molecular, atomic, and nuclear theory meet
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Quadrupole moments of Cd and Zn nuclei: When solid-state, molecular, atomic, and nuclear theory meet. / Haas, Heinz; Sauer, Stephan P. A.; Hemmingsen, Lars Bo Stegeager; Kellö, Vladimir; Zhao, Pengwei W.
I: EPL, Bind 117, Nr. 6, 62001, 2017.Publikation: Bidrag til tidsskrift › Tidsskriftartikel › Forskning › fagfællebedømt
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TY - JOUR
T1 - Quadrupole moments of Cd and Zn nuclei: When solid-state, molecular, atomic, and nuclear theory meet
AU - Haas, Heinz
AU - Sauer, Stephan P. A.
AU - Hemmingsen, Lars Bo Stegeager
AU - Kellö, Vladimir
AU - Zhao, Pengwei W.
PY - 2017
Y1 - 2017
N2 - The nuclear quadrupole moment (Q) of the 5/2+ isomeric state of 111Cd, of particular importance to the interpretation of Perturbed Angular Correlation experiments in condensed matter, was determined by combining existing PAC data with high-level ab initio (CCSD(T)) calculations for Cd-dimethyl and hybrid density functional theory for metallic Cd. A revised value of Q = .641(25) b is found, much reduced from earlier estimates. Using the new result together with the values for other Cd isotopes from atomic data, also recently revised, the trend of Q for the 11/2- states in Cd is in perfect agreement with new nuclear covariant density functional theory calculations. Similar theoretical work for metallic Zn and the ZnS molecule, combined with atomic calculations, also results in an equivalent reduction for the reference value of the 67Zn 5/2-ground state quadrupole moment to Q = .125(5) b.
AB - The nuclear quadrupole moment (Q) of the 5/2+ isomeric state of 111Cd, of particular importance to the interpretation of Perturbed Angular Correlation experiments in condensed matter, was determined by combining existing PAC data with high-level ab initio (CCSD(T)) calculations for Cd-dimethyl and hybrid density functional theory for metallic Cd. A revised value of Q = .641(25) b is found, much reduced from earlier estimates. Using the new result together with the values for other Cd isotopes from atomic data, also recently revised, the trend of Q for the 11/2- states in Cd is in perfect agreement with new nuclear covariant density functional theory calculations. Similar theoretical work for metallic Zn and the ZnS molecule, combined with atomic calculations, also results in an equivalent reduction for the reference value of the 67Zn 5/2-ground state quadrupole moment to Q = .125(5) b.
U2 - 10.1209/0295-5075/117/62001
DO - 10.1209/0295-5075/117/62001
M3 - Journal article
VL - 117
JO - Lettere Al Nuovo Cimento
JF - Lettere Al Nuovo Cimento
SN - 0295-5075
IS - 6
M1 - 62001
ER -
ID: 176862968