2022 roadmap on low temperature electrochemical CO2 reduction

Publikation: Bidrag til tidsskrift › Review › Forskning › fagfællebedømt

Standard

2022 roadmap on low temperature electrochemical CO2 reduction. / Stephens, Ifan E. L.; Chan, Karen; Bagger, Alexander; Boettcher, Shannon W.; Bonin, Julien; Boutin, Etienne; Buckley, Aya K.; Buonsanti, Raffaella; Cave, Etosha R.; Chang, Xiaoxia; Chee, See Wee; da Silva, Alisson H. M.; de Luna, Phil; Einsle, Oliver; Endrodi, Balazs; Escudero-Escribano, Maria; de Araujo, Jorge V. Ferreira; Figueiredo, Marta C.; Hahn, Christopher; Hansen, Kentaro U.; Haussener, Sophia; Hunegnaw, Sara; Huo, Ziyang; Hwang, Yun Jeong; Janaky, Csaba; Jayathilake, Buddhinie S.; Jiao, Feng; Jovanov, Zarko P.; Karimi, Parisa; Koper, Marc T. M.; Kuhl, Kendra P.; Lee, Woong Hee; Liang, Zhiqin; Liu, Xuan; Ma, Sichao; Ma, Ming; Oh, Hyung-Suk; Robert, Marc; Cuenya, Beatriz Roldan; Rossmeisl, Jan; Roy, Claudie; Ryan, Mary P.; Sargent, Edward H.; Sebastian-Pascual, Paula; Seger, Brian; Steier, Ludmilla; Strasser, Peter; Varela, Ana Sofia; Vos, Rafael E.; Wang, Xue; Xu, Bingjun; Yadegari, Hossein; Zhou, Yuxiang.

I: JPhys Energy, Bind 4, Nr. 4, 042003, 01.10.2022.

Publikation: Bidrag til tidsskrift › Review › Forskning › fagfællebedømt

Harvard

Stephens, IEL, Chan, K, Bagger, A, Boettcher, SW, Bonin, J, Boutin, E, Buckley, AK, Buonsanti, R, Cave, ER, Chang, X, Chee, SW, da Silva, AHM, de Luna, P, Einsle, O, Endrodi, B, Escudero-Escribano, M, de Araujo, JVF, Figueiredo, MC, Hahn, C, Hansen, KU, Haussener, S, Hunegnaw, S, Huo, Z, Hwang, YJ, Janaky, C, Jayathilake, BS, Jiao, F, Jovanov, ZP, Karimi, P, Koper, MTM, Kuhl, KP, Lee, WH, Liang, Z, Liu, X, Ma, S, Ma, M, Oh, H-S, Robert, M, Cuenya, BR, Rossmeisl, J, Roy, C, Ryan, MP, Sargent, EH, Sebastian-Pascual, P, Seger, B, Steier, L, Strasser, P, Varela, AS, Vos, RE, Wang, X, Xu, B, Yadegari, H & Zhou, Y 2022, '2022 roadmap on low temperature electrochemical CO2 reduction', JPhys Energy, bind 4, nr. 4, 042003. https://doi.org/10.1088/2515-7655/ac7823

APA

Stephens, I. E. L., Chan, K., Bagger, A., Boettcher, S. W., Bonin, J., Boutin, E., Buckley, A. K., Buonsanti, R., Cave, E. R., Chang, X., Chee, S. W., da Silva, A. H. M., de Luna, P., Einsle, O., Endrodi, B., Escudero-Escribano, M., de Araujo, J. V. F., Figueiredo, M. C., Hahn, C., ... Zhou, Y. (2022). 2022 roadmap on low temperature electrochemical CO2 reduction. JPhys Energy, 4(4), [042003]. https://doi.org/10.1088/2515-7655/ac7823

Vancouver

Stephens IEL, Chan K, Bagger A, Boettcher SW, Bonin J, Boutin E o.a. 2022 roadmap on low temperature electrochemical CO2 reduction. JPhys Energy. 2022 okt. 1;4(4). 042003. https://doi.org/10.1088/2515-7655/ac7823

Author

Stephens, Ifan E. L. ; Chan, Karen ; Bagger, Alexander ; Boettcher, Shannon W. ; Bonin, Julien ; Boutin, Etienne ; Buckley, Aya K. ; Buonsanti, Raffaella ; Cave, Etosha R. ; Chang, Xiaoxia ; Chee, See Wee ; da Silva, Alisson H. M. ; de Luna, Phil ; Einsle, Oliver ; Endrodi, Balazs ; Escudero-Escribano, Maria ; de Araujo, Jorge V. Ferreira ; Figueiredo, Marta C. ; Hahn, Christopher ; Hansen, Kentaro U. ; Haussener, Sophia ; Hunegnaw, Sara ; Huo, Ziyang ; Hwang, Yun Jeong ; Janaky, Csaba ; Jayathilake, Buddhinie S. ; Jiao, Feng ; Jovanov, Zarko P. ; Karimi, Parisa ; Koper, Marc T. M. ; Kuhl, Kendra P. ; Lee, Woong Hee ; Liang, Zhiqin ; Liu, Xuan ; Ma, Sichao ; Ma, Ming ; Oh, Hyung-Suk ; Robert, Marc ; Cuenya, Beatriz Roldan ; Rossmeisl, Jan ; Roy, Claudie ; Ryan, Mary P. ; Sargent, Edward H. ; Sebastian-Pascual, Paula ; Seger, Brian ; Steier, Ludmilla ; Strasser, Peter ; Varela, Ana Sofia ; Vos, Rafael E. ; Wang, Xue ; Xu, Bingjun ; Yadegari, Hossein ; Zhou, Yuxiang. / 2022 roadmap on low temperature electrochemical CO2 reduction. I: JPhys Energy. 2022 ; Bind 4, Nr. 4.

Bibtex

@article{2f7beae865ac414aaea3c776ef063c5a,
title = "2022 roadmap on low temperature electrochemical CO2 reduction",
abstract = "Electrochemical CO2 reduction (CO2R) is an attractive option for storing renewable electricity and for the sustainable production of valuable chemicals and fuels. In this roadmap, we review recent progress in fundamental understanding, catalyst development, and in engineering and scale-up. We discuss the outstanding challenges towards commercialization of electrochemical CO2R technology: energy efficiencies, selectivities, low current densities, and stability. We highlight the opportunities in establishing rigorous standards for benchmarking performance, advances in in operando characterization, the discovery of new materials towards high value products, the investigation of phenomena across multiple-length scales and the application of data science towards doing so. We hope that this collective perspective sparks new research activities that ultimately bring us a step closer towards establishing a low- or zero-emission carbon cycle.",
keywords = "electrocatalysis, CO2 reduction, electrochemistry, solar fuels, CARBON-DIOXIDE CAPTURE, ELECTROCATALYTIC CONVERSION, SELECTIVE ELECTROREDUCTION, TECHNOECONOMIC ANALYSIS, ACCELERATED DISCOVERY, MECHANISTIC INSIGHTS, BIPOLAR MEMBRANES, METAL-ELECTRODES, STRUCTURAL BASIS, LIQUID FUEL",
author = "Stephens, {Ifan E. L.} and Karen Chan and Alexander Bagger and Boettcher, {Shannon W.} and Julien Bonin and Etienne Boutin and Buckley, {Aya K.} and Raffaella Buonsanti and Cave, {Etosha R.} and Xiaoxia Chang and Chee, {See Wee} and {da Silva}, {Alisson H. M.} and {de Luna}, Phil and Oliver Einsle and Balazs Endrodi and Maria Escudero-Escribano and {de Araujo}, {Jorge V. Ferreira} and Figueiredo, {Marta C.} and Christopher Hahn and Hansen, {Kentaro U.} and Sophia Haussener and Sara Hunegnaw and Ziyang Huo and Hwang, {Yun Jeong} and Csaba Janaky and Jayathilake, {Buddhinie S.} and Feng Jiao and Jovanov, {Zarko P.} and Parisa Karimi and Koper, {Marc T. M.} and Kuhl, {Kendra P.} and Lee, {Woong Hee} and Zhiqin Liang and Xuan Liu and Sichao Ma and Ming Ma and Hyung-Suk Oh and Marc Robert and Cuenya, {Beatriz Roldan} and Jan Rossmeisl and Claudie Roy and Ryan, {Mary P.} and Sargent, {Edward H.} and Paula Sebastian-Pascual and Brian Seger and Ludmilla Steier and Peter Strasser and Varela, {Ana Sofia} and Vos, {Rafael E.} and Xue Wang and Bingjun Xu and Hossein Yadegari and Yuxiang Zhou",
year = "2022",
month = oct,
day = "1",
doi = "10.1088/2515-7655/ac7823",
language = "English",
volume = "4",
journal = "JPhys Energy",
issn = "2515-7655",
publisher = "IOP Publishing",
number = "4",

}

RIS

TY - JOUR

T1 - 2022 roadmap on low temperature electrochemical CO2 reduction

AU - Stephens, Ifan E. L.

AU - Chan, Karen

AU - Bagger, Alexander

AU - Boettcher, Shannon W.

AU - Bonin, Julien

AU - Boutin, Etienne

AU - Buckley, Aya K.

AU - Buonsanti, Raffaella

AU - Cave, Etosha R.

AU - Chang, Xiaoxia

AU - Chee, See Wee

AU - da Silva, Alisson H. M.

AU - de Luna, Phil

AU - Einsle, Oliver

AU - Endrodi, Balazs

AU - Escudero-Escribano, Maria

AU - de Araujo, Jorge V. Ferreira

AU - Figueiredo, Marta C.

AU - Hahn, Christopher

AU - Hansen, Kentaro U.

AU - Haussener, Sophia

AU - Hunegnaw, Sara

AU - Huo, Ziyang

AU - Hwang, Yun Jeong

AU - Janaky, Csaba

AU - Jayathilake, Buddhinie S.

AU - Jiao, Feng

AU - Jovanov, Zarko P.

AU - Karimi, Parisa

AU - Koper, Marc T. M.

AU - Kuhl, Kendra P.

AU - Lee, Woong Hee

AU - Liang, Zhiqin

AU - Liu, Xuan

AU - Ma, Sichao

AU - Ma, Ming

AU - Oh, Hyung-Suk

AU - Robert, Marc

AU - Cuenya, Beatriz Roldan

AU - Rossmeisl, Jan

AU - Roy, Claudie

AU - Ryan, Mary P.

AU - Sargent, Edward H.

AU - Sebastian-Pascual, Paula

AU - Seger, Brian

AU - Steier, Ludmilla

AU - Strasser, Peter

AU - Varela, Ana Sofia

AU - Vos, Rafael E.

AU - Wang, Xue

AU - Xu, Bingjun

AU - Yadegari, Hossein

AU - Zhou, Yuxiang

PY - 2022/10/1

Y1 - 2022/10/1

N2 - Electrochemical CO2 reduction (CO2R) is an attractive option for storing renewable electricity and for the sustainable production of valuable chemicals and fuels. In this roadmap, we review recent progress in fundamental understanding, catalyst development, and in engineering and scale-up. We discuss the outstanding challenges towards commercialization of electrochemical CO2R technology: energy efficiencies, selectivities, low current densities, and stability. We highlight the opportunities in establishing rigorous standards for benchmarking performance, advances in in operando characterization, the discovery of new materials towards high value products, the investigation of phenomena across multiple-length scales and the application of data science towards doing so. We hope that this collective perspective sparks new research activities that ultimately bring us a step closer towards establishing a low- or zero-emission carbon cycle.

AB - Electrochemical CO2 reduction (CO2R) is an attractive option for storing renewable electricity and for the sustainable production of valuable chemicals and fuels. In this roadmap, we review recent progress in fundamental understanding, catalyst development, and in engineering and scale-up. We discuss the outstanding challenges towards commercialization of electrochemical CO2R technology: energy efficiencies, selectivities, low current densities, and stability. We highlight the opportunities in establishing rigorous standards for benchmarking performance, advances in in operando characterization, the discovery of new materials towards high value products, the investigation of phenomena across multiple-length scales and the application of data science towards doing so. We hope that this collective perspective sparks new research activities that ultimately bring us a step closer towards establishing a low- or zero-emission carbon cycle.

KW - electrocatalysis

KW - CO2 reduction

KW - electrochemistry

KW - solar fuels

KW - CARBON-DIOXIDE CAPTURE

KW - ELECTROCATALYTIC CONVERSION

KW - SELECTIVE ELECTROREDUCTION

KW - TECHNOECONOMIC ANALYSIS

KW - ACCELERATED DISCOVERY

KW - MECHANISTIC INSIGHTS

KW - BIPOLAR MEMBRANES

KW - METAL-ELECTRODES

KW - STRUCTURAL BASIS

KW - LIQUID FUEL

U2 - 10.1088/2515-7655/ac7823

DO - 10.1088/2515-7655/ac7823

M3 - Review

VL - 4

JO - JPhys Energy

JF - JPhys Energy

SN - 2515-7655

IS - 4

M1 - 042003

ER -

ID: 322645516