Templation and Concentration Drive Conversion between a FeII12L12Pseudoicosahedron, a FeII4L4Tetrahedron, and a FeII2L3Helicate

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Standard

Templation and Concentration Drive Conversion between a FeII12L12Pseudoicosahedron, a FeII4L4Tetrahedron, and a FeII2L3Helicate. / Zhang, Dawei; Gan, Quan; Plajer, Alex J.; Lavendomme, Roy; Ronson, Tanya K.; Lu, Zifei; Jensen, Jesper D.; Laursen, Bo W.; Nitschke, Jonathan R.

I: Journal of the American Chemical Society, Bind 144, 2022, s. 1106-1112.

Publikation: Bidrag til tidsskrift › Tidsskriftartikel › Forskning › fagfællebedømt

Harvard

Zhang, D, Gan, Q, Plajer, AJ, Lavendomme, R, Ronson, TK, Lu, Z, Jensen, JD, Laursen, BW & Nitschke, JR 2022, 'Templation and Concentration Drive Conversion between a FeII12L12Pseudoicosahedron, a FeII4L4Tetrahedron, and a FeII2L3Helicate', Journal of the American Chemical Society, bind 144, s. 1106-1112. https://doi.org/10.1021/jacs.1c11536

APA

Zhang, D., Gan, Q., Plajer, A. J., Lavendomme, R., Ronson, T. K., Lu, Z., Jensen, J. D., Laursen, B. W., & Nitschke, J. R. (2022). Templation and Concentration Drive Conversion between a FeII12L12Pseudoicosahedron, a FeII4L4Tetrahedron, and a FeII2L3Helicate. Journal of the American Chemical Society, 144, 1106-1112. https://doi.org/10.1021/jacs.1c11536

Vancouver

Zhang D, Gan Q, Plajer AJ, Lavendomme R, Ronson TK, Lu Z o.a. Templation and Concentration Drive Conversion between a FeII12L12Pseudoicosahedron, a FeII4L4Tetrahedron, and a FeII2L3Helicate. Journal of the American Chemical Society. 2022;144:1106-1112. https://doi.org/10.1021/jacs.1c11536

Author

Zhang, Dawei ; Gan, Quan ; Plajer, Alex J. ; Lavendomme, Roy ; Ronson, Tanya K. ; Lu, Zifei ; Jensen, Jesper D. ; Laursen, Bo W. ; Nitschke, Jonathan R. / Templation and Concentration Drive Conversion between a FeII12L12Pseudoicosahedron, a FeII4L4Tetrahedron, and a FeII2L3Helicate. I: Journal of the American Chemical Society. 2022 ; Bind 144. s. 1106-1112.

Bibtex

@article{56c3bafa31714697b2183c7b702af01c,
title = "Templation and Concentration Drive Conversion between a FeII12L12Pseudoicosahedron, a FeII4L4Tetrahedron, and a FeII2L3Helicate",
abstract = "We report the construction of three structurally distinct self-assembled architectures: FeII12L12 pseudoicosahedron 1, FeII2L3 helicate 2, and FeII4L4 tetrahedron 3, formed from a single triazatriangulenium subcomponent A under different reaction conditions. Pseudoicosahedral capsule 1 is the largest formed through subcomponent self-assembly to date, with an outer-sphere diameter of 5.4 nm and a cavity volume of 15 nm3. The outcome of self-assembly depended upon concentration, where the formation of pseudoicosahedron 1 was favored at higher concentrations, while helicate 2 exclusively formed at lower concentrations. The conversion of pseudoicosahedron 1 or helicate 2 into tetrahedron 3 occurred following the addition of a CB11H12- or B12F122- template. ",
author = "Dawei Zhang and Quan Gan and Plajer, {Alex J.} and Roy Lavendomme and Ronson, {Tanya K.} and Zifei Lu and Jensen, {Jesper D.} and Laursen, {Bo W.} and Nitschke, {Jonathan R.}",
note = "Publisher Copyright: {\textcopyright} ",
year = "2022",
doi = "10.1021/jacs.1c11536",
language = "English",
volume = "144",
pages = "1106--1112",
journal = "Journal of the American Chemical Society",
issn = "0002-7863",
publisher = "ACS Publications",

}

RIS

TY - JOUR

T1 - Templation and Concentration Drive Conversion between a FeII12L12Pseudoicosahedron, a FeII4L4Tetrahedron, and a FeII2L3Helicate

AU - Zhang, Dawei

AU - Gan, Quan

AU - Plajer, Alex J.

AU - Lavendomme, Roy

AU - Ronson, Tanya K.

AU - Lu, Zifei

AU - Jensen, Jesper D.

AU - Laursen, Bo W.

AU - Nitschke, Jonathan R.

N1 - Publisher Copyright: ©

PY - 2022

Y1 - 2022

N2 - We report the construction of three structurally distinct self-assembled architectures: FeII12L12 pseudoicosahedron 1, FeII2L3 helicate 2, and FeII4L4 tetrahedron 3, formed from a single triazatriangulenium subcomponent A under different reaction conditions. Pseudoicosahedral capsule 1 is the largest formed through subcomponent self-assembly to date, with an outer-sphere diameter of 5.4 nm and a cavity volume of 15 nm3. The outcome of self-assembly depended upon concentration, where the formation of pseudoicosahedron 1 was favored at higher concentrations, while helicate 2 exclusively formed at lower concentrations. The conversion of pseudoicosahedron 1 or helicate 2 into tetrahedron 3 occurred following the addition of a CB11H12- or B12F122- template.

AB - We report the construction of three structurally distinct self-assembled architectures: FeII12L12 pseudoicosahedron 1, FeII2L3 helicate 2, and FeII4L4 tetrahedron 3, formed from a single triazatriangulenium subcomponent A under different reaction conditions. Pseudoicosahedral capsule 1 is the largest formed through subcomponent self-assembly to date, with an outer-sphere diameter of 5.4 nm and a cavity volume of 15 nm3. The outcome of self-assembly depended upon concentration, where the formation of pseudoicosahedron 1 was favored at higher concentrations, while helicate 2 exclusively formed at lower concentrations. The conversion of pseudoicosahedron 1 or helicate 2 into tetrahedron 3 occurred following the addition of a CB11H12- or B12F122- template.

U2 - 10.1021/jacs.1c11536

DO - 10.1021/jacs.1c11536

M3 - Journal article

C2 - 35014803

AN - SCOPUS:85123873914

VL - 144

SP - 1106

EP - 1112

JO - Journal of the American Chemical Society

JF - Journal of the American Chemical Society

SN - 0002-7863

ER -

ID: 291538256