Toward understanding the role of the electric double layer structure and electrolyte effects on well-defined interfaces for electrocatalysis

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Toward understanding the role of the electric double layer structure and electrolyte effects on well-defined interfaces for electrocatalysis. / Sebastian Pascual, Paula; Shao-Horn, Yang ; Escudero Escribano, Maria.

I: Current Opinion in Electrochemistry, Bind 32, 100918, 2022.

Publikation: Bidrag til tidsskrift › Tidsskriftartikel › Forskning › fagfællebedømt

Harvard

Sebastian Pascual, P, Shao-Horn, Y & Escudero Escribano, M 2022, 'Toward understanding the role of the electric double layer structure and electrolyte effects on well-defined interfaces for electrocatalysis', Current Opinion in Electrochemistry, bind 32, 100918. https://doi.org/10.1016/j.coelec.2021.100918

APA

Sebastian Pascual, P., Shao-Horn, Y., & Escudero Escribano, M. (2022). Toward understanding the role of the electric double layer structure and electrolyte effects on well-defined interfaces for electrocatalysis. Current Opinion in Electrochemistry, 32, [100918]. https://doi.org/10.1016/j.coelec.2021.100918

Vancouver

Sebastian Pascual P, Shao-Horn Y, Escudero Escribano M. Toward understanding the role of the electric double layer structure and electrolyte effects on well-defined interfaces for electrocatalysis. Current Opinion in Electrochemistry. 2022;32. 100918. https://doi.org/10.1016/j.coelec.2021.100918

Author

Sebastian Pascual, Paula ; Shao-Horn, Yang ; Escudero Escribano, Maria. / Toward understanding the role of the electric double layer structure and electrolyte effects on well-defined interfaces for electrocatalysis. I: Current Opinion in Electrochemistry. 2022 ; Bind 32.

Bibtex

@article{6186c800cb914afc9b6a4467ce136449,
title = "Toward understanding the role of the electric double layer structure and electrolyte effects on well-defined interfaces for electrocatalysis",
abstract = "The interplay between the structure and composition of the electric double layer and the surface charge controls the electrocatalytic activity of reactions central to decarbonization of chemical fuels and materials. The employed electrolyte can affect the charge distribution and the electric field on the interface, which also alters the local pH and ordering of the water-solvent network. Additionally, the electrolyte plays a key role in stabilizing or destabilizing the adsorbed intermediates via non-covalent bonds, or poisons the surface and induces surface reconstruction, affecting the reactivity of the active sites positions. Herein, we discuss, from an experimental perspective, electrolyte effects on different interfacial properties relevant to electrocatalysis.",
author = "{Sebastian Pascual}, Paula and Yang Shao-Horn and {Escudero Escribano}, Maria",
year = "2022",
doi = "10.1016/j.coelec.2021.100918",
language = "English",
volume = "32",
journal = "Current Opinion in Electrochemistry",
issn = "2451-9103",
publisher = "Elsevier",

}

RIS

TY - JOUR

T1 - Toward understanding the role of the electric double layer structure and electrolyte effects on well-defined interfaces for electrocatalysis

AU - Sebastian Pascual, Paula

AU - Shao-Horn, Yang

AU - Escudero Escribano, Maria

PY - 2022

Y1 - 2022

N2 - The interplay between the structure and composition of the electric double layer and the surface charge controls the electrocatalytic activity of reactions central to decarbonization of chemical fuels and materials. The employed electrolyte can affect the charge distribution and the electric field on the interface, which also alters the local pH and ordering of the water-solvent network. Additionally, the electrolyte plays a key role in stabilizing or destabilizing the adsorbed intermediates via non-covalent bonds, or poisons the surface and induces surface reconstruction, affecting the reactivity of the active sites positions. Herein, we discuss, from an experimental perspective, electrolyte effects on different interfacial properties relevant to electrocatalysis.

AB - The interplay between the structure and composition of the electric double layer and the surface charge controls the electrocatalytic activity of reactions central to decarbonization of chemical fuels and materials. The employed electrolyte can affect the charge distribution and the electric field on the interface, which also alters the local pH and ordering of the water-solvent network. Additionally, the electrolyte plays a key role in stabilizing or destabilizing the adsorbed intermediates via non-covalent bonds, or poisons the surface and induces surface reconstruction, affecting the reactivity of the active sites positions. Herein, we discuss, from an experimental perspective, electrolyte effects on different interfacial properties relevant to electrocatalysis.

U2 - 10.1016/j.coelec.2021.100918

DO - 10.1016/j.coelec.2021.100918

M3 - Journal article

VL - 32

JO - Current Opinion in Electrochemistry

JF - Current Opinion in Electrochemistry

SN - 2451-9103

M1 - 100918

ER -

ID: 288922959